Design, Development and in-vitro evaluation of Herbal Matrix tablet

 

NM Bhopale*, HS Sawarkar1, MB Narkhede1, NV Thorat1, MR Bhise1 and SS Khadabadi2

1I.B.S.S. College of Pharmacy, Malkapur- 443 101 (M.S.)

2 Govt. College of Pharmacy, Amravati-444 603 (M.S.)

 

ABSTRACT

The purpose of the present investigation was to develop the sustain release matrix tablet of Tinospora cordifolia using the various polymers like HPMC (Hydroxy-Propyl-methyl-cellulose), Ethyl cellulose (EC), of different viscosity grade. Ethanolic extract of Tinospora cordifolia was used for the formulation of sustain release matrix tablet and tablet formulations were developed by using wet granulation method. Different diluents like lactose, magnesium stearate and cab-o-sil were used for improving flowability and compressibility. Binder such as polyvinyl pyrrolidone was used for optimization of the formulations. Sodium starch glycolate was used as disintegrating agent. Pre and post formulation parameters were studied for all the batches. HPMC –KM4 shows better result for matrix tablet in terms of sustain drug release with comparison to different viscosity grade of HPMC and ethyl cellulose. The dissolution study of the Tinospora cordifolia tablets exhibited 99.54% release of total polyphenol.

 

KEYWORDS: Ethanolic extract of Tinospora cordifolia, HPMC, Ethyl cellulose, Matrix tablet.

 

INTRODUCTION

Inflammation is the reaction of living tissue to injury, infection, environmental agents, malignancy, and cellular changes. In skin, inflammation is most visible because it causes noticeable swelling, redness, discomfort and pain. The process leading to inflammation, which is known as the inflammatory response, also induces changes that aren't seen but influence the effects of inflammation and their severity1.

 

Studies on induced edema and arthritis and on human arthritis proved the anti-inflammatory potency of the ethanolic extract of this plant. Phase I and Phase II of adjuvant induced arthritis were also inhibited. The anti-inflammatory activity of this plant resembles that of non-steroidal anti-inflammatory agents2. It has weak antipyretic action and is a morphine potentiator. The watery extract of the plant is used as a febrifuge and is called “Indian Quinine”. The plant is used in Ayurvedic rasayanas to improve the immune system and the body's resistance to infections. The bitter principle present shows antiperiodic, antispasmodic, anti-inflammatory and antipyretic properties.3. All the formulation containing Tinospora cordifolia are present in conventional dosage forms which are prone to various problems like fluctuation in drug blood level, patient’s inconvenience, etc.  These problems can be overcome by formulating sustain release tablet using ethanolic extract of Tinospora cordifolia root extract.

 

Material and Methods:

HPMC (K4M, K15M, K100M), Ethyl cellulose (75cps, 100cps), and PVP (K30) were purchased from Loba chem. (Mumbai, India).  Other used chemical were of analytical grade. UV Spectrophotometer (Shimadzu) and tablet punching machine (Rimek minipress) were used for the present study.

 

 


Table no.1) Result of physical constants

Parameters of physical constant

% w/w

1) Total Ash

2) Acid insoluble ash

3) Water soluble Ash

4) Moisture content

6.9 %

4.065 %

5.6 %

6.25 %

Sr. No.

Chemical tests performed

WE

1

Carbohydrates

+

2

Proteins

-

3

Amino acids

-

4

Glycosides

+

 

i)Anthraquinone

+

ii)Cardiac

-

iii)Coumarins

-

iv)Cyanogenetic

-

5

Saponin glycosides

+

6

Alkaloids:

-

7

Flavonoids:

-

8.

Steroids and triterpenoids:

-

9.

Tannins and phenolics

+

10.

Mucilage:

+

11.

Gums:

-

12.

Fixed oil

+

13.

Volatile oil

-

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

Table no. 2) Extractive values of different solvents, with percentage extractability and color of extract

Extract

Extractive value %

Colour of extract

Water soluble extractive

7.6 %

Reddish black

Ethanol soluble extractive

12.26 %

Reddish black

 

Tinospora cordifolia was obtained from local sources and authenticated by Dr. Prabha Y. Bhogaonkar (Director, Government Vidarbha Institute of Science and Humanities, Amravati). Tinospora cordifolia root was extracted by using ehanol as solvent. Preliminary physicochemical parameters and photochemical test of the Tinospora  cordifolia extract (Table no.1, 2) were carried out. Same extract was used for the formulation. The total polyphenol in extract was estimated by Folin Ciocalteu method using UV Spectrophotometer 4.

 

Formulations of Tinospora cordifolia extract 5:

Tablets of Tinospora cordifolia root extract were prepared by wet granulation method. PVP-K30 (10%) and sodium starch glycolate was added as binder and disintegrating agent respectively. Matrix tablet were prepared by using different viscosity grade HPMC and Ethyl cellulose. (Table no.3).

 

The extract, lactose and the polymer were passed through 60# sieve and then granulated using PVP K-30 in isopropyl alcohol as granulating agent, the wet mass was passed through 8# sieve. Granules were air dried for one hour and dried granules were passed through 16# sieve. These granules were lubricated in poly bag using talc and cab-o-sil. Desired quantity of granules were weighed and fed manually to compression machine. The flat faced punch i.e. upper punch with break line and plane lower punch of diameter 10 mm was used for compression.

 

Evaluation of Tinospora cordifolia tablet 6:

The tablets of Tinospora cordifolia extract were prepared by wet granulation method and   evaluated for preformulation parameters such as angle of repose, total porosity, Carr’s index, bulk density, tap density and postformulation parameters like friability, weight variation, hardness, disintegration were measured. (Table no.4)

 

In-Vitro dissolution study of Tinospora cordifolia tablet 7:

The in vitro release of total polyphenol from formulation batches was carried out in 0.1N HCl for 2 hours and continued in pH 6.8 phosphate buffer for remaining 10 hours. The studies were performed using USP dissolution apparatus II at 37 ± 0.5 °C and 50 rpm. Samples were taken at interval of one hour each and analyzed for drug content at 765 nm. using UV-Spectrophotometer.

 

Dissolution study was carried out for each 6 tablet per batch for 12 hours and drug release study was carried out on the basis of total polyphenol contents.

Table no. 3) Results of phytochemical tests.

 

Table no. 4) Formulation table showing composition of each matrix tablet using various different polymers.

Formulation code.Ţ

Ingredients  (mg)ß

F1

F2

F3

F4

F5

F6

Extract of Tinospora  cordifolia

250

250

250

250

250

250

HPMC-K-M4

32

-

-

-

-

-

HPMC-K-M15

-

32

-

-

-

-

HPMC-K-100M

-

-

32

-

-

-

E.C-75cps

-

-

-

30

-

-

E.C-100cps

-

-

-

-

30

-

S.S.G

12

12

12

12

12

12

PVP-K-30

40

40

40

40

40

40

TALC

10

10

10

10

10

10

CAB-O-SIL

10

10

10

10

10

10

LACTOSE

46

46

46

46

46

77

Tablet weight (mg)

400

400

400

400

400

400

 

Since, polyphenol constitutes the major chemical entity in Tinospora cordifolia; we thought it logical to evaluate our formulation with respect to total polyphenol content.

With respect to total polyphenol contents present in extract, the drug release study was carried out. The results of dissolution study were given in table no. 5.

 

Results and Discussion:

Extractive values such as ethanol soluble extractive value was found to be 12.26% and water soluble extractive value was found 7.6%. Ash values such as total ash, acid insoluble ash, and water soluble ash were found to be 6.9%, 4.065 %, 5.6 % respectively. Moisture content was found to be 6.25%. Total polyphenol content was found to be 41.55% (Table no. 1, 2).

 

Fig. no.1) In vitro release profile of all formulations showing sustains effect for twelve hours.

 

 


Table no. 5) Evaluation parameters of granules.

Parameters →

Formulations ↓

Loose bulk density (LBD)

Tapped bulk density (TBD)

Carr’s index (I)

Angle of Repose (Ө)

Total Porosity

F1

0.506 + 0.02

0.589 +0.036

14.89 +0.95

37.44 +0.12

27.43 +0.03

F2

0.290 +0.03

0.337+ 0.04

14.53 +0.05

37.02 +0.01

37.03 +0.04

F3

0.306 +0.02

0.351 +0.019

11.95 +0.33

37.72 +0.43

34.27 +0.02

F4

0.290 +0.04

0.338 +0.032

14.35 + 0.14

36.56 +0.01

37.03 0+.04

F5

0.309 +0.04

0.354 +0.023

13.11 +0.89

35.75 +1.68

31.25 +0.03

F6

0.509 + 0.002

0.579 +0.008

12.14 +0.94

36.89 +0.58

30.23 +0.02

 

 


Table no. 6) Percent release profiles of formulations of Tinospora cordifolia extract containing HPMC and ethyl cellulose

% released of Drug

Formulation code

Time(hrs)

F1

F2

F3

F4

F5

F6

1

37.97

47.29

34.27

40.84

37.1

63.17

2

45.39

52.49

36.07

44.57

42.55

80.11

3

53.3

55.69

47.43

45.72

51.93

97.54

4

60.36

59.46

49.33

47.43

52.34

_

5

63.17

61.7

53.09

49.12

53.93

_

6

67.07

66.18

53.81

49.72

61.32

_

7

70.99

68.66

54.39

62.42

66.66

_

8

72.73

74.43

58.79

65.43

72.34

_

9

80.11

78.5

59.9

70.13

82.86

_

10

80.14

95.61

60.46

72.85

83.05

_

11

83.79

97.36

61.11

73.01

86.25

_

12

97.54

97.38

70.1

73.04

87.09

_

 

Phytochemical study ethanol extract of Tinospora cordifolia were shows presence of carbohydrates, glycosides, anthraquinone, saponin glycosides, tannins and phenolics, mucilage and fixed oil (Table no. 3).

 

Since, polyphenol constitute are major chemical entity in Tinospora cordifolia, we thought it logical to evaluate our formulation with respect to total polyphenol content. Polyphenol content can be taken as a reliable and reproducible parameter for the dissolution study of the Tinospora cordifolia formulation.

 

In the current research work an attempt was made to formulate a matrix tablet of Tinospora cordifolia extract. From the results it can be concluded that, the matrix tablet prepared using by using ethanolic extracts of Tinospora cordifolia is found to be a novel one. Sustain release matrix tablets of Tinospora cordifolia were prepared successfully using EC and HPMC as release retarding polymers by wet granulation method (Table no 4). Various evaluation parameter for the granules like bulk density, tap density, angle of repose, total porosity and Carr’s index suggest that granules has good flow property (Table no 5). Various evaluation parameters for tablets like thickness, hardness, friability and disintegration of all formulations were found to be satisfactory. In case of formulations containing HPMC, viscosity was a major factor affecting the drug release. An inverse relationship existed between polymer viscosity and drug release; thus higher the polymer viscosity lower was the drug release. From the dissolution study it was found that HPMC K4M shows better drug release, as compared to other polymers (Table no 6).

 

CONCLUSION:

Present research work deals with the formulation and evaluation of matrix tablet. Tinospora cordifolia root were purchased from the local market of Nagpur.

Dr. Prabha Y. Bhogaonkar, Director, Vidarbha Institute of Science and Humanities had done the authentication of Tinospora cordifolia Linn.

 

Various Physical parameters like,  Total ash, Water soluble ash, Acid insoluble ash, LOD, Water soluble extractive value, Ethanol soluble extractive value of Tinospora cordifolia were determined.

Various qualitative tests for inorganic elements like Aluminum, Chloride, and Copper etc. were determined.

 

Ethanolic extract of root of Tinospora cordifolia was prepared and this extract was tested for presence of various Phytochemicals like Carbohydrates, Proteins, Alkaloids, Glycosides, etc.

 

Formulations were prepared by using ethanol root extract of Tinospora cordifolia and various sustained release polymers.

 

The granules were prepared by using Wet granulation method and evaluated for various parameters i.e. Bulk density, % Compressibility index, Angle of repose and Total porosity. These granules were then compressed into tablet and evaluated for various parameters i.e. Thickness, Hardness, Weight variation, Friability, Disintegration time. All these formulations passed the criteria of IP.

 

In case of formulations containing HPMC, viscosity was a major factor affecting the drug release. An inverse relationship existed between polymer viscosity and drug release; thus higher the polymer viscosity lower was the drug release.

 

From the results it can be concluded that, the Matrix Tablet prepared using extracts of Tinospora  cordifolia is found to be a novel one.

 

References:

1)       R. S. Satoskar, S. D. Bhandarkar, Pharmacology and pharmacotherapeutics, 9th edition, Popular prakashan, Mumbai, page 159-160

2)       Pendse, V. K., M. M. Mahawar, N. K. Khanna, K. C. Somani and S. K. Gautam, Anti-inflammatory and related activity of water extract of Tinospora cordifolia, 1981, Indian Drugs 19, 1, 14--21.

3)       Dr. K.M. Nadkarni, The Indian Materia Medica, Vol.I, pg 1220-1221

4)       Quality standards of Indian medicinal plants.  Vol-1 Indian Council of Medicinal Research, New Delhi 2003, page 208-211, 42-46.

5)       James Swarbrick, James C. Boylan, Controlled and Modified-Release Drug-   Delivery system, Encyclopedia of Pharmaceutical Technology, vol-3, page 281-315.

6)       Leon Lachman, Herbert A. Liberrman, Joseph L. Kanig, the Theory and Practice of Industrial Pharmacy, 3rd edition, Varghese Publishing House, page 298-301, 302, 320, 325-329.

7)       Murina Momin, A. F. Amin and K. Pundarikakshudu, Development and Evaluation of Triphala Formulations, Indian J. pharm. Sci., 2004, 66(4): 427-432.

 

Received on 04.09.2009

Accepted on 07.11.2009        

© A&V Publication all right reserved

Research Journal of Pharmaceutical Dosage Forms and Technology. 1(3): Nov. – Dec. 2009, 254-256